Nano-structured Thin Films for Hydrogen-Permeation Barrier Applied on AISI 1018 Steel Used in Petroleum Applications

Mohammed, Neam F.; Mahdi, Bahaa S.; Thamir, Amin D.

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Nano-structured Thin Films for Hydrogen-Permeation Barrier Applied on AISI 1018 Steel Used in Petroleum Applications

Engineering and Technology Journal

Article 1, Volume 41, Issue 6, Spring 2023, Page 1-12 PDF (1143 K)

Document Type: Research Paper

DOI: 10.30684/etj.2022.134357.1268

Authors

Neam F. Mohammed¹; Bahaa S. Mahdi

²; Amin D. Thamir³

¹University of Technology - Department of Production Engineering and Metallurgy - Metallurgy Branch

²University of Technology-Iraq / Production and Metallurgy Engineering Department / Metallurgy Branch

³University of Technology - Department of Production Engineering and Metallurgy

Abstract

Hydrogen embrittlement is a diffusible Hydrogen that is harmful to the toughness of iron. It follows, therefore, that the harmful influence of diffusible Hydrogen can be mitigated by preventing its entry into steel. This approach was achieved by usingthree coating layersas a coating nanostructure thin layer by DC sputtering on steel structural (AISI l018) and hydrogen charging (HC) effect on uncoated and different Nano coated tensile specimens. The first layer was Titanium as a bonding layer, the second layer was TiO₂ with Al₂O₃, and the third layer was Al₂O₃. Using a titanium Nano layer coating on AISI1018 steel tensile specimens increased the tensile strength from 570 to 659 MPa with 16 hours of charging, which is considered a good increase. In contrast, the elongation remained in a steady-state with little difference in values compared to changing the charging time and the coating of the double layer. Furthermore, it was found that samples coated with TiO₂ and Al₂O₃ by the DC method had advanced hydrogen embrittlement resistance and increased tensile strength (from 565 to 680 MPa with 8 hours of charging process). Moreover, the maximum adhesion value was related to the triple layer at 596 psi, and the lowest value was 309 psi using the titanium layer alone. The coating time was 5 hours of the sputtering process for all specimens. Thecoating layers are considered a good barrier for hydrogen permeation through steel structures (AISI 1018).

Highlights

A third coating layer gives an acceptable adhesion force with the highest deposition rate.
Nano-structured coating increased bulk AISI 1018 steel tensile strength after the hydrogen charging process.
Double layer of Ti and TiO2+Al2O3 coat gives a 20 percent increase in tensile strength after HC for AISI 1018 steel.
The layer of ceramic coatings TiO2with Al₂O₃ as coating Nano-structured thin films can improve the hydrogen permeation resistance .
The Nano titanium layer showed the main portion in bonding.

Keywords

DC sputtering; hydrogen permeation; hot filament Hydrogen charging; Nano-structured; hydrogen embrittlement

References

[1] R.N. Iyer, H.W. Pickering, Mechanism and kinetics of electrochemical hydrogen entry and degradation of metallic systems. Annu Rev Mater Sci. 20 (1990) 299-338. https://doi.org/10.1146/annurev.ms.20.080190.001503

[2] R.P. Gangloff, Critical issues in hydrogen assisted cracking of structural alloys, Oxford Elsevier Science. 1 (2008) 141-165.https://doi.org/10.1016/B978-008044635-6.50015-7

[3] M. M. Mirza, E. Rasu, A. Desilva, Influence of Nano additives on Protective Coatings for Oil Pipe Lines of Oman, Int. J. Chem. Eng. Appl. 7 (2016) 221-224. https://doi: 10.18178/ijcea.2016.7.4.577

[4] M. J. Kadhim, K. A. Sukkar, Investigation Nano coating for Corrosion Protection of Petroleum Pipeline Steel Type A106 Grade B. Theoretical and Practical Study in Iraqi Petroleum Sector, Eng. Technol. J. 35 (2017) 1042- 3413.

[5] Q. J. Sulaiman, A. Al – Taie, D.M. Hassan, Evaluation of Sodium Chloride and Acidity Effect on Corrosion of Buried Carbon Steel Pipeline in Iraqi Soil, Iraqi J. Chem. Pet. Eng. 15 (2014) 1-8.https://doi.org/10.31699/IJCPE

[6] C. Matteo, Current and Future Nanotech Applications in the Oil Industry, Am. J. Appl. Sci., 9 (2012) 784-793. https://doi.org/10.3844/ajassp.2012.784.793

[7] T. Michler, J. Naumann, Influence of high-pressure hydrogen on the tensile and fatigue properties of a high strength Cu–Al–Ni–Fe alloy”, Int. J. Hydrogen Energy 35 (2010). https://doi.org/10.1016/j.ijhydene.2010.07.093

[8] G. Balakrishnan, Effect of substrate temperature on microstructure and properties of nano crystalline titania thin films prepared by pulsed laser deposition nano systems, physics, chemistry, mathematics, 7 (2016) 621–623. http://dx.doi.org/10.17586/2220-8054-2016-7-4-621-623

[9] H.J. Cialone and J.H. Holbrook. Sensitivity of Steels to Degradation in Gaseous Hydrogen, In: Hydrogen Embrittlement: Prevention and Control, ASTM STP 962, L. Raymond (Ed.), , pp. 134-152, 1988. https://doi.10.1520/STP45297S

[10] A. Barnoush,H.Vehoff, Recent developments in the study of hydrogen embrittlement: Hydrogen effect on dislocation nucleation. Acta Mater, 58 (2010) 5274-5285. https://doi.org/10.1016/j.actamat.2010.05.057

[11] J. Song, W.A. Curtin, Atomic mechanism and prediction of hydrogen embrittlement in iron. Nat Mater. 12 (2013) 145–151 . https://doi.org/10.1038/nmat3479

[12] H.K. Birnbaum, Hydrogen effects on deformation and fracture, science and sociology. MRS Bull. 28 (2003) 479-485. https://doi.org/10.1557/mrs2003.143

[13] M. Dadfarnia, P. Novak, D. C. Ahn, J. B. Liu, P. Sofronis, D. D. Johnson at all. Recent advancesin the study of structural materials compatibility with hydrogen. Adv Mater, 22 (2010) 1128-1135. https://doi.org/10.1002/adma.200904354

[14] Y. Katz, N. Tymiak, W.W. Gerberich, Nanomechanical probes as new approaches to hydrogen/deformation interaction studies. Engng Fract Mech, 68 (2001) 619-646.https://doi.org/10.1016/S0013-7944(00)00119-3

[15] Gerberich WW, Marsh PG, Hoehn JW. Hydrogen induced cracking mechanisms. In: Moody NR, Hoehn JW, editors. Hydrogen effects in materials. Warrendale, PA: TMS, 1996.

[16] H. M. Jedy, R.A. Anaee, Characterization of Nb2O5-Ni Coating Prepared by DC Sputtering, Eng. Technol. J. 39 (2021) 565-572. https://doi.org/10.30684/etj.v39i4A.1902

[17] A. Shanaghi, A. S.Rouhaghdam, M. Aliofkhazraei, Study of TiO₂ nanoparticle coatings by the SOL-GEL methods for corrosion protection, Mater. Sci. 44 (2008) 233-246. https://doi.10.1007/s11003-008-9070-6

[18] M.A. Deyab, S.T. Keer, Effect of nano-TiO2 particles size on the corrosion resistance of alkyd coating. Materials Chemistry and Physics journal homepage: Elsevier, 146 (2014) 406-411. https://doi.org/10.1016/j.matchemphys.2014.03.045

[19] T.Eguchi, M.Tamura, Nanostructured thin films for hydrogen-permeation barrier, Journal of Vacuum Science & Technology A: Vacuum, Surfaces, and Films,33 (2015)041503. https://doi.org/10.1116/1.4919736

[20] X. Li ,L.Chen, H. Liu,C. Shi, D. Wang ,Z. Mi and L.Qiao, Prevention of Hydrogen Damage Using MoS2 Coating on Iron Surface, Nanomaterials 9 (2019) 1-10. https://doi.org/10.3390/nano9030382

[21] M.Wasim, M. B. Djukic, Hydrogen embrittlement of low carbon structural steel at macro-, micro- and nano-levels. Int. J. Hydrog. Energy. 45 (2020) 2145-2156.https://doi.org/10.1016/j.ijhydene.2019.11.070

[22] Autoren, C. Wegst, M. Wegst, "Key to steel",part 1, 2004.

[23] ASTM E8-04 " Standard Test Methods for Tension Testing of Metallic Materials". American Association State. 2010.

[24] D. L. Liu, J. Martin, and N. A. Burnham, Optimal roughness for minimal adhesion, Appl. Phys. Lett. 91 (2007) 043107.https://doi.org/10.1063/1.2763981

[25] S. Ayadi, Y. Charles, M. Gaspérini, I. C.Lemaire, T. D. S. Botelho, Effect of loading mode on blistering in iron submitted to plastic prestrain before hydrogen cathodic charging, Int. J. Hydrog. Energy.42 (2017) 10555-10567 https://doi.org/10.1016/j.ijhydene.2017.02.048

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